Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.
Tracking Ultrafast Charge Separation in a PBI-based Biomimetic Complex for Oxygen Evolution / Maiuri, Margherita; Russo, Mattia; Moretti, Luca; Petropoulos, Vasilis; Rigodanza, Francesco; Sartorel, Andrea; Prato, Maurizio; Cerullo, Giulio; Bonchio, Marcella. - (2020), pp. M4B.10-M4B.13. ( The 22nd International Conference on Ultrafast Phenomena 2020 Washington D.C. USA ) [10.1364/UP.2020.M4B.10].
Tracking Ultrafast Charge Separation in a PBI-based Biomimetic Complex for Oxygen Evolution
Moretti, Luca;
2020-01-01
Abstract
Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.
